>>> Any tips/recommendations for starting?

Well, don't install software just for the sake of installing software.

That is, if you need synchronization between your devices, then look for software that will solve your problem. In this example Syncthing will solve your problem. But, if you don't need to have synchronization - don't just install some software.

If you need any specific software for a specific task, don't hesitate to ask.

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Discussion

My only problem with Syncthing and KDE Connect is that all devices need to visible on your LAN. If your devices are running a VPN this can trip up connectivity locally.

It's not a problem at all. Play with your firewall settings.

I'm under a VPN right now, but on the LAN all my devices communicate with each other fine. :)

I'll have a look at it tomorrow. Thanks.